That fallout map is just a time-captured example - a snapshot, if you will.
We ran much more detailed versions, using global weather data compiled every 6 hours, modeled at different altitudes for plume intercept by the fleet of WC-130s, WC-135s, B-52s, and U-2s. Using that variety of airframes, collection was planned from essentially 1,500 feet to the operational limits of the U-2/TR-1. Even the old BUFF could stairstep up to 50K ft, but it protested mightily enroute. NASA had their two WB-57 Canberras that could also assist to 60K+ feet, if needed.
Once intercept was established, we reported plume size, heading, altitude, and intensity. They took that data and updated the models and forecasts, with particular emphasis given to population centers in the projected path.
IOW, if Wright-Patterson got nuked, how soon would the greater Chicago area be at risk, etc.